A Robust, Biodegradable, and Fire‐Retardant Cellulose Nanofibers‐Based Structural Material Fabricated from Natural Sargassum

D De‐Han Li (Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China) Z Zi‐Meng Han (Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China) M Meng Shao (Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China) Z Zhi‐Jin Jiao (Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China) C Chen Gao (Department of Physics, Xiamen University) W Wen‐Bin Sun (Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China) Z Zhao‐Xiang Liu (Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China) K Kun‐Peng Yang (Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China) Q Qing‐Fang Guan (Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China) S Shu‐Hong Yu (New Cornerstone Science Laboratory Department of Chemistry Institute of Biomimetic Materials and Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials and Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China)

Abstract

Abstract With increasing concern about the environmental pollution of petrochemical plastics, people are constantly exploring environmentally friendly and sustainable alternative materials. Compared with petrochemical materials, cellulose has overwhelming superiority in terms of mechanical properties, thermal properties, cost, and biodegradability. However, the flammability of cellulose hinders its practical application to a certain extent, so improving the fire‐retardant properties of cellulose nanofiber‐based materials has become a research focus. Here, cellulose nanofiber and alginate are extracted from abundant natural sargassum as high‐strength nanoscale building blocks, and then a sargassum cellulose fire‐retardant structural material is prepared through a bottom‐up hydrogel layer‐by‐layer method. The structural materials obtained incorporate excellent mechanical properties (≈297 MPa), thermal stability (≈200 °C), low thermal expansion coefficient (≈7.17 × 10 −6 K −1 ), and fire‐retardant properties. This work largely improves the utilization of seaweed residue and natural polymers, providing a bio‐based fire‐retardant strategy, and has a wide range of development prospects in the field of fiber‐based high‐performance structural materials in the future.

Article Details

Volume / Issue Vol. 37, Issue 9
Published March 01, 2025
ISSN 0935-9648
Publisher Unknown Publisher

Journal Info

Advanced Materials

Unknown Publisher

ISSN: 0935-9648 Physical Sciences

Authors (10)

D

De‐Han Li

Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China

Z

Zi‐Meng Han

Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China

M

Meng Shao

Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China

Z

Zhi‐Jin Jiao

Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China

C

Chen Gao

Department of Physics, Xiamen University

W

Wen‐Bin Sun

Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China

Z

Zhao‐Xiang Liu

Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China

K

Kun‐Peng Yang

Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China

Q

Qing‐Fang Guan

Department of Chemistry New Cornerstone Science Laboratory Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China

S

Shu‐Hong Yu

New Cornerstone Science Laboratory Department of Chemistry Institute of Biomimetic Materials and Chemistry Anhui Engineering Laboratory of Biomimetic Materials Division of Nanomaterials and Chemistry Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 China