Designing Moderately‐Solvating Electrolytes for High‐Performance Lithium–Sulfur Batteries

D David J. Kautz (Energy and Environment Directorate Pacific Northwest National Laboratory Richland WA 99354 USA) X Xia Cao P Peiyuan Gao (Pacific Northwest National Laboratory) S Shuo Feng (State Key Laboratory of Precision and Intelligent Chemistry, School of Chemistry and Materials Science) Q Qian Zhao (Zhejiang University , , ,) S Saurabh Parab (Department of Nano Engineering University of California San Diego La Jolla CA 92093 USA) Y Yaobin Xu J Joseph P. Quinn (Energy and Environment Directorate Pacific Northwest National Laboratory Richland WA 99354 USA) M Muhammad Mominur Rahman (Chemistry Division Brookhaven National Laboratory Upton NY 11973 USA) S Sha Tan (Hangzhou Institute of Advanced Studies, Zhejiang Normal University 1 , 1108 Gengwen Road, Hangzhou 311231, Zhejiang Province,) X Xin Zhang S Sanaz Ketabi (General Motors Research and Development Center Warren MI 48092 USA) A Aqsa Nazir (Energy and Environment Directorate Pacific Northwest National Laboratory Richland WA 99354 USA) J Junxia Wang F Fang Dai S Shen Wang D Dongping Lu (School of Agriculture and Biology, Shanghai Jiao Tong University) E Enyuan Hu (Chemistry Division) Y Y. Shirley Meng (Department of Nano Engineering University of California San Diego La Jolla CA 92093 USA) C Chongmin Wang J Jun Liu J Ji‐Guang Zhang (Energy and Environment Directorate Pacific Northwest National Laboratory Richland Washington USA) W Wu Xu (State Key Laboratory of Precision and Intelligent Chemistry, School of Chemistry and Materials Science)

Abstract

Abstract New electrolytes are critical for high‐energy lithium (Li)–sulfur (S) batteries (LSBs) to ensure their stability against Li metal anode and polysulfides (PSs) shuttling which hinder the large‐scale application of LSBs. In this study, the design principle of moderately solvating electrolytes (MSEs) for LSBs is demonstrated by using a multiple‐solvent system comprising of a highly solvating solvent, a weakly solvating solvent, and a non‐solvating solvent to create a well‐balanced electrolyte system. This resulting electrolyte significantly improves the cycle life of LSBs, achieving 300 cycles, which is twice as long as that of similar cells with the conventional electrolyte and it also ensures stable calendar life for at least seven months. The optimal MSE forms robust passivation layers enhancing the structural integrity of both S and Li metal electrodes after cycling. These virtues effectively hinder parasitic side reactions and self‐discharge behavior of LSBs. This electrolyte design principle is versatile and can be applied to other battery chemistries, providing a potential path toward the development of a more efficient and stable battery system. By addressing key challenges such as the instability of electrodes and shuttling of polysulfides, this electrolyte approach offers promising solutions for advancing LSB technology.

Article Details

Volume / Issue Vol. 37, Issue 33
Published August 01, 2025
ISSN 0935-9648
Publisher Unknown Publisher

Journal Info

Advanced Materials

Unknown Publisher

ISSN: 0935-9648 Physical Sciences

Authors (23)

D

David J. Kautz

Energy and Environment Directorate Pacific Northwest National Laboratory Richland WA 99354 USA

X

Xia Cao

P

Peiyuan Gao

Pacific Northwest National Laboratory

S

Shuo Feng

State Key Laboratory of Precision and Intelligent Chemistry, School of Chemistry and Materials Science

Q

Qian Zhao

Zhejiang University , , ,

S

Saurabh Parab

Department of Nano Engineering University of California San Diego La Jolla CA 92093 USA

Y

Yaobin Xu

J

Joseph P. Quinn

Energy and Environment Directorate Pacific Northwest National Laboratory Richland WA 99354 USA

M

Muhammad Mominur Rahman

Chemistry Division Brookhaven National Laboratory Upton NY 11973 USA

S

Sha Tan

Hangzhou Institute of Advanced Studies, Zhejiang Normal University 1 , 1108 Gengwen Road, Hangzhou 311231, Zhejiang Province,

X

Xin Zhang

S

Sanaz Ketabi

General Motors Research and Development Center Warren MI 48092 USA

A

Aqsa Nazir

Energy and Environment Directorate Pacific Northwest National Laboratory Richland WA 99354 USA

J

Junxia Wang

F

Fang Dai

S

Shen Wang

D

Dongping Lu

School of Agriculture and Biology, Shanghai Jiao Tong University

E

Enyuan Hu

Chemistry Division

Y

Y. Shirley Meng

Department of Nano Engineering University of California San Diego La Jolla CA 92093 USA

C

Chongmin Wang

J

Jun Liu

J

Ji‐Guang Zhang

Energy and Environment Directorate Pacific Northwest National Laboratory Richland Washington USA

W

Wu Xu

State Key Laboratory of Precision and Intelligent Chemistry, School of Chemistry and Materials Science