Hierarchical MoS <sub>2</sub> /Poly(ionic liquid) Metamaterials for Electrically Tunable Terahertz Stealth

Y Yujie Zhong F Fuwei Sun (Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing, School of Mechanical Engineering and Automation) S Shuncong Zhong Y Yi Huang (Hubei Cancer Hospital Wuhan China) J Jiewen Lin (Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China) Q Qiukun Zhang Y Yaosen Deng (Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China) T Tingling Lin (Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China) Q Qiuming Zeng (Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China) Y Yonglin Huang (Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China) J Jianfeng Zhong (Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China) C Chenglong Guan (Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China) S Shantung Tu (School of Mechanical and Power Engineering East China University of Science and Technology Shanghai 200237 P. R. China) M Minghong Wu (School of Environmental and Chemical Engineering)

Abstract

Abstract Active absorption modulation is critical for advanced stealth technologies, especially given the emerging detection threat from terahertz atmospheric windows. However, due to the difficulty in balancing high absorption and tunability, the actual manufacturing of most terahertz absorbers usually neglects the integration of electrical tuning, which limits their development of dynamic wave trapping for electronic countermeasure systems. Here, a terahertz stealth metamaterial (TSM) with hierarchical ionotronic architecture is proposed to overcome the tradeoff. Large‐area continuous MoS 2 assemblies tightly attached poly(ionic liquid) (PIL) microarrays provide enough conditions for surface electron conduction and plasmon mode excitation. By establishing wave‐electron‐ion interaction pathways, the directional migration of free anions inside the PIL and the accumulation of excess charge carriers up to 100.4% at the MoS 2 interfaces are promoted, thereby stimulating changes in the plasma frequency of the absorption system. Consequently, this micro‐nano structural design enhances the absorption tunability and combines multiple dissipative behaviors. TSM exhibit high specific attenuation (−275 dB mm −1 ), frequency agility (21.4%), and phase switching (153.1 deg.) within terahertz atmospheric windows. Moreover, the template‐assisted assembly strategy adopted has the potential to be used for the building of universal blocks operating within other frequency ranges.

Article Details

Volume / Issue Vol. 37, Issue 37
Published September 01, 2025
ISSN 0935-9648
Publisher Unknown Publisher

Journal Info

Advanced Materials

Unknown Publisher

ISSN: 0935-9648 Physical Sciences

Authors (14)

Y

Yujie Zhong

F

Fuwei Sun

Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing, School of Mechanical Engineering and Automation

S

Shuncong Zhong

Y

Yi Huang

Hubei Cancer Hospital Wuhan China

J

Jiewen Lin

Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China

Q

Qiukun Zhang

Y

Yaosen Deng

Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China

T

Tingling Lin

Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China

Q

Qiuming Zeng

Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China

Y

Yonglin Huang

Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China

J

Jianfeng Zhong

Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China

C

Chenglong Guan

Fujian Provincial Key Laboratory of Terahertz Functional Devices and Intelligent Sensing School of Mechanical Engineering and Automation Fuzhou University Fuzhou 350108 P. R. China

S

Shantung Tu

School of Mechanical and Power Engineering East China University of Science and Technology Shanghai 200237 P. R. China

M

Minghong Wu

School of Environmental and Chemical Engineering