Michell's‐Instability‐Mediated Fast Reconfiguration of Hydrogel‐Based Ring Actuators

Q Qing Li Zhu (Department of Polymer Science and Engineering Ministry of Education Key Laboratory of Macromolecular Synthesis and Functionalization Zhejiang University Hangzhou 310058 China) Z Zhijie Li (Molecular Medicine Program, The Hospital for Sick Children) H Hanlei Cheng (Department of Polymer Science and Engineering Ministry of Education Key Laboratory of Macromolecular Synthesis and Functionalization Zhejiang University Hangzhou 310058 China) W Weixuan Liu (School of Physical Science and Technology Shanghai Tech University Shanghai China) Z Zhi Jian Wang (Institute for Chemical Reaction Design and Discovery (WPI-ICReDD)) O Olena Khoruzhenko (Bavarian Polymer Institute and Department of Chemistry University of Bayreuth Universitätsstrasse 30 95440 Bayreuth Germany) J Josef Breu (Department of Chemistry, University of Bayreuth, Universitätsstraße 30, 95447 Bayreuth, Germany) W Wei Hong Q Qiang Zheng Z Zi Liang Wu

Abstract

Abstract Michell's instability, a classic type of mechanical instability, has received tremendous interest from different disciplines. It occurs when the pre‐torsion in an elastic ring surpasses a critical value; the elastic ring spontaneously undergoes a transition from a flat or warped shape to a figure‐of‐eight configuration. However, such instability has rarely been exploited in designing soft actuators. Here, by employing a stimulus‐triggered Michell's instability, hydrogel‐based ring actuators capable of fast shape morphing are developed. Upon heating or light irradiation, the hydrogel ring transforms rapidly from the saddle‐shape into the figure‐of‐eight configuration. Rigorous experiments and simulations reveal the underlying mechanism and attribute it to the stimuli‐induced variations in bending and torsional stiffnesses of the gel string with anisotropic structure and response, which reduces the critical twist for Michell's instability of the ring actuator. Moreover, effects of light intensity, environmental temperature, ring size, and pre‐torsion on reconfiguration are also investigated. The fast action of the ring actuators in aqueous conditions has been demonstrated through various tasks, such as screwing a bottle cap, kicking a ball, and triggering synergetic deformations. The design principle of soft actuators by harnessing Michell's instability should merit the development of other soft machines with fast action and large‐amplitude reconfiguration.

Article Details

Volume / Issue Vol. 38, Issue 7
Published February 01, 2026
ISSN 0935-9648
Publisher Unknown Publisher

Journal Info

Advanced Materials

Unknown Publisher

ISSN: 0935-9648 Physical Sciences

Authors (10)

Q

Qing Li Zhu

Department of Polymer Science and Engineering Ministry of Education Key Laboratory of Macromolecular Synthesis and Functionalization Zhejiang University Hangzhou 310058 China

Z

Zhijie Li

Molecular Medicine Program, The Hospital for Sick Children

H

Hanlei Cheng

Department of Polymer Science and Engineering Ministry of Education Key Laboratory of Macromolecular Synthesis and Functionalization Zhejiang University Hangzhou 310058 China

W

Weixuan Liu

School of Physical Science and Technology Shanghai Tech University Shanghai China

Z

Zhi Jian Wang

Institute for Chemical Reaction Design and Discovery (WPI-ICReDD)

O

Olena Khoruzhenko

Bavarian Polymer Institute and Department of Chemistry University of Bayreuth Universitätsstrasse 30 95440 Bayreuth Germany

J

Josef Breu

Department of Chemistry, University of Bayreuth, Universitätsstraße 30, 95447 Bayreuth, Germany

W

Wei Hong

Q

Qiang Zheng

Z

Zi Liang Wu