Molecular Engineering of Polymer Brushes Enables Lithium–Sulfur Battery Stable Operation under Ultra‐Wide Temperature Range

B Borui Li (School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)) W Wanyuan Jiang (State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, School of Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)) Y Yunpeng Qu (School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)) W Wenkai Song X Xin Jin M Mengfan Pei (School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)) S Shuo Zhuo (School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)) R Runyue Mao (School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)) L Lin Wang D Dongming Liu (School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)) X Xigao Jian (School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)) F Fangyuan Hu (School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province))

Abstract

Abstract Achieving stable operation under a wide temperature range is a critical target for the practical applications of lithium–sulfur batteries. However, intense lithium polysulfides (LiPSs) shuttling at high‐temperature, sluggish sulfur species conversion, and inhomogeneous Li + deposition at low‐temperature severely impair the cycle lifespan of batteries. Herein, the multifunctional polymer brushes are fabricated by grafting anthraquinone‐functionalized poly(glycidyl methacrylate) brushes on graphene surfaces (G‐pGMAAQ) to simultaneously regulate the evolution of sulfur and lithium species. Combining theoretical calculations and experiments, it is revealed that G‐pGMAAQ serves as a redox mediator that reduces the LiPSs conversion energy barrier, and its unique polar brush‐like structure effectively inhibits LiPSs shuttling and homogenizes Li + flow. Hence, G‐pGMAAQ facilitates lithium–sulfur batteries stable operation in an ultra‐wide temperature range (−40–70 °C). Furthermore, the Ah‐level pouch cell achieves an energy density of 417 Wh kg −1 , demonstrating the commercial potential of polymer brushes for lithium–sulfur batteries.

Article Details

Volume / Issue Vol. 37, Issue 35
Published September 01, 2025
ISSN 0935-9648
Publisher Unknown Publisher

Journal Info

Advanced Materials

Unknown Publisher

ISSN: 0935-9648 Physical Sciences

Authors (12)

B

Borui Li

School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)

W

Wanyuan Jiang

State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, School of Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)

Y

Yunpeng Qu

School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)

W

Wenkai Song

X

Xin Jin

M

Mengfan Pei

School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)

S

Shuo Zhuo

School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)

R

Runyue Mao

School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)

L

Lin Wang

D

Dongming Liu

School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)

X

Xigao Jian

School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)

F

Fangyuan Hu

School of Materials Science and Engineering, State Key Laboratory of Fine Chemicals, Frontiers Science Center for Smart Materials Oriented Chemical Engineering, Technology Innovation Center of High Performance Resin Materials (Liaoning Province)