Multidimensional Photopatterning of Heterogeneous Liquid‐Crystal Superstructures Toward Higher‐Level Information Optics

S Si‐Jia Liu (National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation College of Engineering and Applied Sciences and Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China) Y Yi‐Heng Zhang (National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation College of Engineering and Applied Sciences and Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China) R Rui Sun P Peng Chen L Lin Zhu D Dong Zhu W Wen Chen (Department of Immunology, St. Jude Children’s Research Hospital) Y Yi‐Ming Wang (National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation College of Engineering and Applied Sciences and Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China) S Shi‐Hui Ding (National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation College of Engineering and Applied Sciences and Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China) S Shi‐Jun Ge (National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation College of Engineering and Applied Sciences and Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China) W Wei Hu Y Yan‐Qing Lu (National Laboratory of Solid State Microstructures & Collaborative Innovation Center of Advanced Microstructures & College of Engineering and Applied Sciences Nanjing University Nanjing China)

Abstract

Abstract Soft matter, featuring superior flexibility and intriguing tunability, has shown enormous potential in sensors, soft robots, and light tailoring. However, limited by its inherent structural complexity, soft matter remains uncompetitive in multidimensional and high‐density information optics. Herein, a heterogeneous liquid‐crystal (LC) superstructure composed of interlocked nematic and chiral LCs is designed to achieve higher‐dimensional light control. Optically multidimensional photopatterning with programmable UV polarization and dosage is proposed to precisely customize both transverse and longitudinal LC arrangements, bringing in a wide range of light‐matter interactions within a single micrometer‐thick film. The constructed heterogeneous LC superstructure not only enables simultaneous near‐field full‐color printing and far‐field full‐color holography but also boasts brightness controllability and polarization selectivity. This low‐cost photonic structure enables a high information density of ≈1.6 million hybrid‐dimensional optical data per square millimeter, unlocking new capabilities in optical storage, display, and encryption. This work creates an ingenious bond between advanced photopatterning technologies and higher‐level optical informatics, and pioneers soft‐matter‐mediated full‐dimensional optics.

Article Details

Volume / Issue Vol. 37, Issue 37
Published September 01, 2025
ISSN 0935-9648
Publisher Unknown Publisher

Journal Info

Advanced Materials

Unknown Publisher

ISSN: 0935-9648 Physical Sciences

Authors (12)

S

Si‐Jia Liu

National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation College of Engineering and Applied Sciences and Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China

Y

Yi‐Heng Zhang

National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation College of Engineering and Applied Sciences and Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China

R

Rui Sun

P

Peng Chen

L

Lin Zhu

D

Dong Zhu

W

Wen Chen

Department of Immunology, St. Jude Children’s Research Hospital

Y

Yi‐Ming Wang

National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation College of Engineering and Applied Sciences and Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China

S

Shi‐Hui Ding

National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation College of Engineering and Applied Sciences and Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China

S

Shi‐Jun Ge

National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation College of Engineering and Applied Sciences and Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China

W

Wei Hu

Y

Yan‐Qing Lu

National Laboratory of Solid State Microstructures & Collaborative Innovation Center of Advanced Microstructures & College of Engineering and Applied Sciences Nanjing University Nanjing China