Orbital Topology of Chiral Crystals for Orbitronics

K Kenta Hagiwara (Peter Grünberg Institut (PGI‐6) Forschungszentrum Jülich 52425 Jülich Germany) Y Ying‐Jiun Chen (Peter Grünberg Institut (PGI‐6) Forschungszentrum Jülich 52425 Jülich Germany) D Dongwook Go (Institute of Physics, Johannes Gutenberg-University Mainz, Mainz, Germany.) X Xin Liang Tan (Peter Grünberg Institut (PGI‐6) Forschungszentrum Jülich 52425 Jülich Germany) S Sergii Grytsiuk K Kui‐Hon Ou Yang (Department of Physics National Taiwan University Taipei 10617 Taiwan) G Guo‐Jiun Shu (Department of Materials and Mineral Resources Engineering National Taipei University of Technology Taipei 10608 Taiwan) J Jing Chien (Department of Physics National Taiwan University Taipei 10617 Taiwan) Y Yi‐Hsin Shen (Department of Physics National Taiwan University Taipei 10617 Taiwan) X Xiang‐Lin Huang (Department of Materials and Mineral Resources Engineering National Taipei University of Technology Taipei 10608 Taiwan) I Iulia Cojocariu (Peter Grünberg Institut (PGI‐6) Forschungszentrum Jülich 52425 Jülich Germany) V Vitaliy Feyer (Peter Grünberg Institute (PGI‐6) Jülich Research Center Jülich Germany) M Minn‐Tsong Lin (Department of Physics National Taiwan University Taipei 10617 Taiwan) S Stefan Blügel C Claus Michael Schneider (Peter Grünberg Institut (PGI‐6) Forschungszentrum Jülich 52425 Jülich Germany) Y Yuriy Mokrousov (Institute of Physics, Johannes Gutenberg-University Mainz, Mainz, Germany.) C Christian Tusche (Peter Grünberg Institut (PGI-6), Forschungszentrum Jülich 1 , 52425 Jülich,)

Abstract

Abstract Chirality is ubiquitous in nature and manifests in a wide range of phenomena including chemical reactions, biological processes, and quantum transport of electrons. In quantum materials, the chirality of fermions, given by the relative directions between the electron spin and momentum, is connected to the band topology of electronic states. This study shows that in structurally chiral materials like CoSi, the orbital angular momentum (OAM) serves as the main driver of a nontrivial band topology in this new class of unconventional topological semimetals, even when spin‐orbit coupling is negligible. A nontrivial orbital‐momentum locking of multifold chiral fermions in the bulk leads to a pronounced OAM texture of the helicoid Fermi arcs at the surface. The study highlights the pivotal role of the orbital degree of freedom for the chirality and topology of electron states, in general, and paves the way towards the application of topological chiral semimetals in orbitronic devices.

Article Details

Volume / Issue Vol. 37, Issue 27
Published July 01, 2025
ISSN 0935-9648
Publisher Unknown Publisher

Journal Info

Advanced Materials

Unknown Publisher

ISSN: 0935-9648 Physical Sciences

Authors (17)

K

Kenta Hagiwara

Peter Grünberg Institut (PGI‐6) Forschungszentrum Jülich 52425 Jülich Germany

Y

Ying‐Jiun Chen

Peter Grünberg Institut (PGI‐6) Forschungszentrum Jülich 52425 Jülich Germany

D

Dongwook Go

Institute of Physics, Johannes Gutenberg-University Mainz, Mainz, Germany.

X

Xin Liang Tan

Peter Grünberg Institut (PGI‐6) Forschungszentrum Jülich 52425 Jülich Germany

S

Sergii Grytsiuk

K

Kui‐Hon Ou Yang

Department of Physics National Taiwan University Taipei 10617 Taiwan

G

Guo‐Jiun Shu

Department of Materials and Mineral Resources Engineering National Taipei University of Technology Taipei 10608 Taiwan

J

Jing Chien

Department of Physics National Taiwan University Taipei 10617 Taiwan

Y

Yi‐Hsin Shen

Department of Physics National Taiwan University Taipei 10617 Taiwan

X

Xiang‐Lin Huang

Department of Materials and Mineral Resources Engineering National Taipei University of Technology Taipei 10608 Taiwan

I

Iulia Cojocariu

Peter Grünberg Institut (PGI‐6) Forschungszentrum Jülich 52425 Jülich Germany

V

Vitaliy Feyer

Peter Grünberg Institute (PGI‐6) Jülich Research Center Jülich Germany

M

Minn‐Tsong Lin

Department of Physics National Taiwan University Taipei 10617 Taiwan

S

Stefan Blügel

C

Claus Michael Schneider

Peter Grünberg Institut (PGI‐6) Forschungszentrum Jülich 52425 Jülich Germany

Y

Yuriy Mokrousov

Institute of Physics, Johannes Gutenberg-University Mainz, Mainz, Germany.

C

Christian Tusche

Peter Grünberg Institut (PGI-6), Forschungszentrum Jülich 1 , 52425 Jülich,