Self‐Cooling Molecular Spin Qudits

E Elias Palacios (Instituto de Nanociencia y Materiales de Aragón (INMA), CSIC & Universidad de Zaragoza) D David Aguilà (Departament de Química Inorgànica i Orgànica, and IN2UB Universitat de Barcelona Diagonal 645 Barcelona 08028 Spain) D David Gracia (Instituto de Nanociencia y Materiales de Aragón (INMA)) D Diamatoula Maniaki (Departament de Química Inorgànica i Orgànica, and IN2UB Universitat de Barcelona Diagonal 645 Barcelona 08028 Spain) L Leoní A. Barrios (Departament de Química Inorgànica i Orgànica Universitat de Barcelona Diagonal 645 Barcelona 08028 Spain) A Alessandro Chiesa (Department of Mathematical, Physical and Computer Sciences) J Jesús I. Martínez (Instituto de Nanociencia y Materiales de Aragón (INMA) CSIC‐Universidad de Zaragoza and Departamento de Física de la Materia Condensada Universidad de Zaragoza Zaragoza 50009 Spain) V Valentin Novikov (Departament de Química Inorgànica i Orgànica Universitat de Barcelona Diagonal 645 Barcelona 08028 Spain) O Olivier Roubeau (Instituto de Nanociencia y Materiales de Aragón (INMA) CSIC and Universidad de Zaragoza Plaza San Francisco s/n Zaragoza 50009 Spain) S Stefano Carretta (Department of Mathematical, Physical and Computer Sciences) M Marco Evangelisti (Instituto de Nanociencia y Materiales de Aragón (INMA)) G Guillem Aromí (Departament de Química Inorgànica i Orgànica Universitat de Barcelona Diagonal 645 Barcelona 08028 Spain) F Fernando Luis (Instituto de Nanociencia y Materiales de Aragón (INMA) CSIC‐Universidad de Zaragoza and Departamento de Física de la Materia Condensada Universidad de Zaragoza Zaragoza 50009 Spain)

Abstract

Abstract The need of operating molecular spin qubits at very low temperatures constitutes a technological limitation. This challenge is addressed by integrating, in the same material and at the molecular scale, quantum processing and magnetic refrigeration capabilities. The molecular unit is a [GdEr] heterolanthanide coordination complex, where Er(III) encodes a qubit while Gd(III) provides a large magnetocaloric effect. The properties of each component are separately studied in isostructural [LaEr] and [GdLu] complexes, where each functional ion lies next to a diamagnetic metal. All complexes are characterized by magnetic, heat capacity, and EPR measurements. The results show that the presence of both ions in the same molecule has a synergic effect on both functionalities. Thus, the coupling between Er(III) and Gd(III) spins lifts any level degeneracies even close to zero magnetic field, leading to a d = 16 set of spin states that, as revealed by pulse EPR measurements, can be coherently manipulated. In turn, Er(III) enhances the magnetocaloric effect compared to [GdLu], extending it to lower temperatures. This is corroborated by direct magnetocaloric measurements, which show the ability of this material to cool itself, and a device, down to temperatures as low as 0.4 K.

Article Details

Volume / Issue Vol. 1, Issue 1
Published October 21, 2025
ISSN 0935-9648
Publisher Unknown Publisher

Journal Info

Advanced Materials

Unknown Publisher

ISSN: 0935-9648 Physical Sciences

Authors (13)

E

Elias Palacios

Instituto de Nanociencia y Materiales de Aragón (INMA), CSIC & Universidad de Zaragoza

D

David Aguilà

Departament de Química Inorgànica i Orgànica, and IN2UB Universitat de Barcelona Diagonal 645 Barcelona 08028 Spain

D

David Gracia

Instituto de Nanociencia y Materiales de Aragón (INMA)

D

Diamatoula Maniaki

Departament de Química Inorgànica i Orgànica, and IN2UB Universitat de Barcelona Diagonal 645 Barcelona 08028 Spain

L

Leoní A. Barrios

Departament de Química Inorgànica i Orgànica Universitat de Barcelona Diagonal 645 Barcelona 08028 Spain

A

Alessandro Chiesa

Department of Mathematical, Physical and Computer Sciences

J

Jesús I. Martínez

Instituto de Nanociencia y Materiales de Aragón (INMA) CSIC‐Universidad de Zaragoza and Departamento de Física de la Materia Condensada Universidad de Zaragoza Zaragoza 50009 Spain

V

Valentin Novikov

Departament de Química Inorgànica i Orgànica Universitat de Barcelona Diagonal 645 Barcelona 08028 Spain

O

Olivier Roubeau

Instituto de Nanociencia y Materiales de Aragón (INMA) CSIC and Universidad de Zaragoza Plaza San Francisco s/n Zaragoza 50009 Spain

S

Stefano Carretta

Department of Mathematical, Physical and Computer Sciences

M

Marco Evangelisti

Instituto de Nanociencia y Materiales de Aragón (INMA)

G

Guillem Aromí

Departament de Química Inorgànica i Orgànica Universitat de Barcelona Diagonal 645 Barcelona 08028 Spain

F

Fernando Luis

Instituto de Nanociencia y Materiales de Aragón (INMA) CSIC‐Universidad de Zaragoza and Departamento de Física de la Materia Condensada Universidad de Zaragoza Zaragoza 50009 Spain