Advanced Materials
Articles in this Issue
Ultra‐Flexible Pixelated Perovskite Photodetectors Enabled by Honeycomb Polymer Grids for High‐Resolution Imaging
AbstractA nature‐inspired fabrication method based on a photolithography‐free flexible polymer grid is reported for high‐resolution pixelation of perovskite photodiode arrays with exceptional mechanic...
A Polymeric mRNA Vaccine Featuring Enhanced Site‐Specific mRNA Delivery and Inherent STING‐Stimulating Performance for Tumor Immunotherapy
AbstractThe development of mRNA delivery carriers with innate immune stimulation functions has emerged as a focal point in the field of mRNA vaccines. Nonetheless, the expression of mRNA in specific s...
High Cell to Module Efficiency Remaining Ratio of ≈90% for the 100 cm<sup>2</sup> Fully Roll‐to‐Roll Gravure Printed Flexible Organic Solar Cells From Non‐Halogenated Solvent
AbstractThe cell‐to‐module (CTM) efficiency remaining ratio from monolithic device to large‐area module indicates the scalability potential for large‐area organic solar cells (OSCs). Nowadays, the CTM...
Electromagnetically Heating and Oscillating Liquid Metal for Catalyzing Polyester Depolymerization
Abstract Depolymerization and recycling of polyesters have shown great significance to economy, ecology, carbon neutrality and human health. Efficient catalysts...
Integrating Strong Luminescence and High Mobility in Organic Single Crystals of Covalent Pyrene Dimers
AbstractSimultaneously achieving strong luminescence and high mobility in organic semiconductors remains a challenge. Herein, two covalently dimerized pyrene derivatives (1Py‐2Py and 1Py‐1Py) with dis...
Multi‐Objective Optimization of Ionic Polymer Electrolytes for High‐Voltage Fast‐Charging and Versatile Lithium Batteries
Abstract Designing ionic polymer electrolytes (IPEs) for high‐voltage and fast‐charging lithium batteries involves searching in a highly complex and discrete che...
Orbital Angular Momentum Correlated Charge to Spin Conversion in Metallic Antiferromagnet
AbstractCurrent‐induced spin‐orbit torque (SOT) allows efficient electrical manipulation on magnetization in spintronic devices. Maximizing the SOT efficiency is a key goal that is pursued via increas...
Anion Vacancies Coupling with Heterostructures Enable Advanced Aerogel Cathode for Ultrafast Aqueous Zinc‐Ion Storage
Abstract As a potential cathode material, manganese‐based sulfide has recently attracted increasing interest due to its many advantages in aqueous zinc‐ion stora...
Metalloenzyme‐Inspired Cluster Fabrication within Mesoporous Channels Featuring Optimized Catalytic Microenvironments for Efficient Neutral pH H <sub>2</sub> O <sub>2</sub> Electrosynthesis
Abstract In nature, some metalloenzymes facilitate highly efficient catalytic transformations of small molecules, primarily attributed to the effective coupling...
Blue Perovskite Light‐Emitting Diodes Using Multifunctional Small Molecule Dopants
Abstract Unbalanced charge carrier injections and high densities of non‐radiative recombination channels are still major obstacles to advancing high‐efficiency b...
Exploring the Mechanisms of Charge Transfer and Identifying Active Sites in the Hydrogen Evolution Reaction Using Hollow C@MoS<sub>2</sub>‐Au@CdS Nanostructures as Photocatalysts
AbstractPlasmonic metal–semiconductor nanocomposites are promising candidates for considerably enhancing the solar‐to‐hydrogen conversion efficiency of semiconductor‐based photocatalysts across the en...
Triplet State Suppression for Energy Loss Reduction in 20% Nonhalogenated Solvent Processed Binary Organic Solar Cells
AbstractBoosting power conversion efficiency (PCE) of organic solar cells (OSCs) has been restricted by its undesirably high energy loss, especially for those nonhalogenated solvent‐processed ones. He...
An Adaptive Solid‐State Synapse with Bi‐Directional Relaxation for Multimodal Recognition and Spatio‐Temporal Learning
Abstract The brain's unique processing power, such as perception, understanding, and interaction with the multimodal world, is achieved through diverse synaptic functionalities, whic...
High‐Entropy Metal Sulfide Nanocrystal Libraries for Highly Reversible Sodium Storage
AbstractControlled synthesis of high‐entropy materials offers a unique platform to explore unprecedented electrochemical properties. High‐entropy metal sulfides (HEMSs) have recently emerged as promis...
Formulation and Characterization of Novel Ionizable and Cationic Lipid Nanoparticles for the Delivery of Splice‐Switching Oligonucleotides
AbstractDespite increasing knowledge about the mechanistic aspects of lipid nanoparticles (LNPs) as oligonucleotide carriers, the structure‐function relationship in LNPs has been generally overlooked....
Manipulating Molecular Stacking for Semitransparent Organic Photovoltaics Achieving Light Utilization Efficiency >6%
Abstract The trade‐off between average visible transmittance (AVT) and power conversion efficiency (PCE), governed by the molecular stacking of the donor and acc...
Smart Polydimethylsiloxane Materials: Versatility for Electrical and Electronic Devices Applications
AbstractBio‐inspired autonomous smart polydimethylsiloxane (PDMS) and its composite materials hold immense promise for a wide range of applications in electrical and electronic devices. These material...
Rejuvenation of Tumor‐Specific T Cells via Ultrahigh DAR Antibody‐Polymeric Imidazoquinoline Complexes: Coordinated Targeting of PDL1 and Efficient TLR7/8 Activation in Intratumoral Dendritic Cells
AbstractIntratumoral dendritic cells (DCs) are pivotal in tumor treatment due to their immature and pro‐tumoral state induced by the tumor microenvironment. Clinically, these immature DCs correlate wi...
High‐Entropy High‐Temperature High‐Piezoelectricity Ceramics
Abstract High‐temperature piezoelectric materials are essential components of transducers and accelerometers applied in the fields of aircraft engines, automobil...
Gradient‐Metasurface‐Contact Photodetector for Visible‐to‐Near‐Infrared Spin Light
AbstractSpin light detection is a rapidly advancing field with significant impact on diverse applications in biology, medicine, and photonics. Developing integrated circularly polarized light (CPL) de...
Core/Shell‐Structured Carbon Support Boosting Fuel Cell Durability
Abstract To enhance the lifetime of proton exchange membrane fuel cells, developing highly durable platinum‐based cathode catalysts is essential. While two degra...
In Situ Cross‐Linking and Interfacial Engineering via Multifunctional Diamine Additive for High‐Temperature Magnesium Metal Batteries
AbstractThe electrolyte and its interfacial chemistry are crucial for the development of high‐temperature magnesium metal batteries. Here, a robust in situ cross‐linked gel polymer electrolyte (MgB@CG...
Atomically Dispersed Co/Mo Sites Anchored on Mesoporous Carbon Hollow Spheres for Highly Selective Oxygen Reduction to Hydrogen Peroxide in Acidic Media
Abstract Two‐electron oxygen reduction reaction (2e − ORR) in acidic media is a promising route for the decentralized and...
Proximity‐Mediated Multi‐Ferroelectric Coupling in Highly Strained EuO‐Graphene Heterostructures
Abstract2D van der Waals materials and their heterostructures are a fantastic playground to explore emergent phenomena arising from electronic quantum hybridization effects. In the last decade, the sp...
Porous Silicon Nanoneedles Efficiently Deliver Adenine Base Editor to Correct a Recurrent Pathogenic <i>COL7A1</i> Variant in Recessive Dystrophic Epidermolysis Bullosa
Abstract Base editing, a CRISPR‐based genome editing technology, enables precise correction of single‐nucleotide variants, promising resolutive treatment for mon...